摘要
Thehighharmonicgeneration(HHG)fromtheCS2moleculeinintenselaserfieldsisinvestigatedusingtheextendedLewensteinmethod.Tileinitialstateisthehighest-occupiedmolecularorbitaloftheCS2molecule,whichcanbewelldescribedbyGaussianwavepacketusingGAMESS-UKpackage.Comparedwiththecaseoftheellipticallaser,theHHGcanbeextendedintwo-colorcircularlypolarizedlaserfield.Thetime-frequencyanalysisandclassicalelectrontrajectoryaswellastheionizationyieldcurvearealsopresentedtofurtherexplaintheunderlyingmechanism.Afteraddingastaticelectricfieldonthez-direction,thesinglequantumpathcontrolisrealizedandthesupercontinuumspectraareobtained.Moreover,anisolated110aspulsecanbeobtainedbysuperposingtheharmonicsfrom130thto1SOthorder.
出版日期
2017年01月11日(中国期刊网平台首次上网日期,不代表论文的发表时间)